Angle-resolved RABBIT: new work and presentation

Angle-resolved RABBIT: new work and presentation

The above image shows simulated velocity map images (left, middle) and angle and time-resolved measurements (right) for angle-resolved RABBIT measurements. In this type of measurement, XUV and IR pulses are combined, and create a set of 1 and 2-photon bands in the photoelectron spectrum. The presence of multiple interfering pathways to each final photoelectron band (energy) results in complex and information rich interferograms, with both angle and time-dependence.

A manuscript detailing this work is currently in preparation, and a recent presentation detailing some aspects of the work can be found on Figshare.

Update 24th March – new manuscript, Angle-resolved RABBIT: theory and numerics, pre-print available.

Time-resolved multi-mass ion imaging: femtosecond UV-VUV pump-probe spectroscopy with the PImMS camera

Time-resolved multi-mass ion imaging: femtosecond UV-VUV pump-probe spectroscopy with the PImMS camera

UPDATE: Dec. 2017

The figure above has made it as the JCP Christmas card!

The  full JCP special issue on Velocity Map Imaging Techniques is also now officially ready, see this page, or this PDF, for all the details.

UPDATE: 4th April 2017

The article is now published in the Journal of Chemical Physics, with an accompanying press release, The Inner Lives of Molecules, from AIP.

The full dataset and analysis scripts are now also available via OSF, DOI: 10.17605/OSF.IO/RRFK3.

Feb. 2017 – new article on the arXiv:

Time-resolved multi-mass ion imaging: femtosecond UV-VUV pump-probe spectroscopy with the PImMS camera

The Pixel-Imaging Mass Spectrometry (PImMS) camera allows for 3D charged particle imaging measurements, in which the particle time-of-flight is recorded along with (x,y) position. Coupling the PImMS camera to an ultrafast pump-probe velocity-map imaging spectroscopy apparatus therefore provides a route to time-resolved multi-mass ion imaging, with both high count rates and large dynamic range, thus allowing for rapid measurements of complex photofragmentation dynamics. Furthermore, the use of vacuum ultraviolet wavelengths for the probe pulse allows for an enhanced observation window for the study of excited state molecular dynamics in small polyatomic molecules having relatively high ionization potentials. Herein, preliminary time-resolved multi-mass imaging results from C2F3I photolysis are presented. The experiments utilized femtosecond UV and VUV (160.8~nm and 267~nm) pump and probe laser pulses in order to demonstrate and explore this new time-resolved experimental ion imaging configuration. The data indicates the depth and power of this measurement modality, with a range of photofragments readily observed, and many indications of complex underlying wavepacket dynamics on the excited state(s) prepared.

arXiv 1702.00744 (2017)

Now published in JCP:
The Journal of Chemical Physics 147, 013911 (2017);
DOI: http://dx.doi.org/10.1063/1.4978923

Also on Authorea, DOI: 10.22541/au.149030711.19068540

 

 

Scientific imaging with the Lytro lightfield camera

Scientific imaging with the Lytro lightfield camera

The Lytro digital camera introduces a Shack-Hartmann configuration into a digital SLR camera.  Why?  For “lightfield” (wavefront) imaging, allowing for depth information in the captured data.  While this kind of thing has long been used for scientific instruments, in particular for laser beam measurements, the Lytro camera brings this capability (and the not insignificant post-processing know-how and hardware required) to photography in the visible.  For rather more detailed information, check out the PhD thesis of Ren Ng, the founder of Lytro.

Here’s a demo image of our VIRP chamber, note that mousing around the image and clicking allows one to change the focus of the image, and the imaging plane.  Mouse wheel to zoom.  It’s going to be an excellent tool for scientific imaging!

* Banner image from Lytro.com.

Reading today…

Reading today…

Quantum imaging with undetected photons

Gabriela Barreto Lemos, Victoria Borish, Garrett D. Cole, Sven Ramelow, Radek Lapkiewicz & Anton Zeilinger

Nature 512, 409–412 (2014)

doi:10.1038/nature13586

Interferometric imaging based on photon pairs, from the intro:

Information is central to quantum mechanics. In particular, quantum interference occurs only if there exists no information to distinguish between the superposed states. The mere possibility of obtaining information that could distinguish between overlapping states inhibits quantum interference1, 2. Here we introduce and experimentally demonstrate a quantum imaging concept based on induced coherence without induced emission3, 4. Our experiment uses two separate down-conversion nonlinear crystals (numbered NL1 and NL2), each illuminated by the same pump laser, creating one pair of photons (denoted idler and signal). If the photon pair is created in NL1, one photon (the idler) passes through the object to be imaged and is overlapped with the idler amplitude created in NL2, its source thus being undefined. Interference of the signal amplitudes coming from the two crystals then reveals the image of the object. The photons that pass through the imaged object (idler photons from NL1) are never detected, while we obtain images exclusively with the signal photons (from NL1 and NL2), which do not interact with the object. Our experiment is fundamentally different from previous quantum imaging techniques, such as interaction-free imaging5 or ghost imaging6, 7, 8, 9, because now the photons used to illuminate the object do not have to be detected at all and no coincidence detection is necessary. This enables the probe wavelength to be chosen in a range for which suitable detectors are not available. To illustrate this, we show images of objects that are either opaque or invisible to the detected photons. Our experiment is a prototype in quantum information—knowledge can be extracted by, and about, a photon that is never detected.